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Thermal and structural studies of Li2O-Na2O-SrO-TiO2-B2O3-P2O5 glasses by DTA, IR and EPR spectroscopy


 
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1. Title Title of document Thermal and structural studies of Li2O-Na2O-SrO-TiO2-B2O3-P2O5 glasses by DTA, IR and EPR spectroscopy
 
2. Creator Author's name, affiliation, country H. Bih; Faculté polydisciplinaire de Taza, Université Sidi Mohamed ben Abdellah, Fes , Morocco.
 
2. Creator Author's name, affiliation, country H. Sinouh; Equipe de Physico-Chimie de la Matière Condensée, PCMC, Faculté des Sciences de Meknes. Université Moulay Ismail, Morocco
 
2. Creator Author's name, affiliation, country H. Es-soufi; Equipe de Physico-Chimie de la Matière Condensée, PCMC, Faculté des Sciences de Meknes. Université Moulay Ismail, Morocco
 
2. Creator Author's name, affiliation, country L. Bih; Equipe de Physico-Chimie de la Matière Condensée, PCMC, Faculté des Sciences de Meknes. Université Moulay Ismail, Morocco
 
2. Creator Author's name, affiliation, country M. Haddad; Laboratoire de Spectrométrie, des Matériaux et Archéomatériaux (LASMAR), Faculté des Sciences de Meknes, Université My Ismail , Morocco
 
2. Creator Author's name, affiliation, country L. Bejjit; Laboratoire de Spectrométrie, des Matériaux et Archéomatériaux (LASMAR), Faculté des Sciences de Meknes, Université My Ismail , Morocco
 
2. Creator Author's name, affiliation, country B. Manoun; Laboratoire des Sciences des Matériaux, des Milieux et de la Modélisation (LS3M), Univ Hassan 1er, 26000, Morocco
 
2. Creator Author's name, affiliation, country P. Lazor; Department of Earth Sciences, Uppsala University, SE-752 36, Uppsala, Sweden
 
3. Subject Discipline(s)
 
3. Subject Keyword(s) borophosphate glasses; thermal analysis; IR; EPR; mixed alkali effect (MAE)
 
4. Description Abstract Glasses in the system 33.33[xNa2O-(1-x)Li2O]-2.5SrO-2.5TiO2-45B2O3-16.67P2O5 (0.0 ≤ x ≤ 1.0) were prepared by standard melt quenching procedures, and their physical properties were characterized by thermal analysis, density measurements. Their local structures were comprehensively characterized by Infrared spectroscopy (IR) and electron paramagnetic resonance (EPR). The variation of the glass transition temperature as a function of the glass compositions is non-linear. The infrared spectroscopy of the glasses has identified the presence of different structural grouping units in the glassy-matrix. It is found that the stretching and bending vibration modes of borate groups are more sensitive to the substitution of alkali elements. EPR experiments have shown the presence of Ti3+ centres in the glasses. The variation of the g-factor as a function of the Na/(Na+Li) ratio presents a minimum around (x=0.5). The composition non-linearity behavior of Tg, vibration bending mode, and g-factor are signature of the mixed alkali effect in the glasses.
 
5. Publisher Organizing agency, location
 
6. Contributor Sponsor(s) The authors would like to thank the Swedish Research Council for the financial support of this work.
 
7. Date (YYYY-MM-DD) 17-08-2017
 
8. Type Status & genre Peer-reviewed Article
 
8. Type Type
 
9. Format File format PDF
 
10. Identifier Uniform Resource Identifier https://revues.imist.ma/index.php/jasi/article/view/9493
 
10. Identifier Digital Object Identifier (DOI) https://doi.org/10.48442/IMIST.PRSM/jasi-v1i1-3.9493
 
11. Source Title; vol., no. (year) Journal of Applied Surfaces and Interfaces; Vol 1, No 1-3 (2017)
 
12. Language English=en en
 
13. Relation Supp. Files
 
14. Coverage Geo-spatial location, chronological period, research sample (gender, age, etc.)
 
15. Rights Copyright and permissions Copyright (c) 2017 Journal of Applied Surfaces and Interfaces