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Synthesis, Structural and Vibrational Studies of Lacunar Apatite type NaPb2CaSr(PO4)3


 
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1. Title Title of document Synthesis, Structural and Vibrational Studies of Lacunar Apatite type NaPb2CaSr(PO4)3
 
2. Creator Author's name, affiliation, country Said Louihi
 
2. Creator Author's name, affiliation, country M'Barek Azdouz
 
2. Creator Author's name, affiliation, country Bouchaib Manoun; Université Hassan 1er; Morocco
 
2. Creator Author's name, affiliation, country Youssef Tamraoui
 
2. Creator Author's name, affiliation, country Abdellah Nia
 
2. Creator Author's name, affiliation, country El mostapha Magha
 
2. Creator Author's name, affiliation, country Jamal Biya
 
2. Creator Author's name, affiliation, country Peter Lazor
 
3. Subject Discipline(s)
 
3. Subject Keyword(s) Lacunar apatite, X-ray diffraction, Rietveld method, Raman spectroscopy
 
4. Description Abstract

NaPb2CaSr(PO4)3 lacunar apatite was synthesized by the solid-state reaction method. The compound was characterized by X-ray diffraction, Raman and infrared spectroscopies. The crystal structure of this new compound has been determined by Rietveld method, adopting the space group P63/m (No. 176), with a=b=9.6684(3)Å and c=7.1104(3)Å The analysis shows that the M(2) sites are shared by four cations Ca, Sr, Pb and Na. While the M(1) sites are occupied by the Ca, Sr and Pb cations. The structure was described as built up from [PO4]3- tetrahedra and Pb2+/Ca2+/Sr2+ of sixfold coordination cavities (6h positions), which delimit void hexagonal tunnels running along [0 0 1]. The tunnels are connected by cations of mixed sites (4f) half occupied by Pb2+/ Ca2+/Sr2+ and half by Na+ mixed alkali cation.

            The results of vibrational spectroscopy are in good agreements with the XRD measurements, the assignments of internal modes of (PO4)3- tetrahedra have been made and corroborate well with factor group analysis for the symmetry P63/m.

An attempt to purify phosphoric acid is done using our apatite and the results are promising.

 
5. Publisher Organizing agency, location
 
6. Contributor Sponsor(s) Swedish Research Council
 
7. Date (YYYY-MM-DD) 19-05-2018
 
8. Type Status & genre Peer-reviewed Article
 
8. Type Type
 
9. Format File format PDF
 
10. Identifier Uniform Resource Identifier https://revues.imist.ma/index.php/jasi/article/view/11215
 
10. Identifier Digital Object Identifier (DOI) https://doi.org/10.48442/IMIST.PRSM/jasi-v3i1-3.11215
 
11. Source Title; vol., no. (year) Journal of Applied Surfaces and Interfaces; Vol 3, No 1-3 (2018)
 
12. Language English=en en
 
13. Relation Supp. Files
 
14. Coverage Geo-spatial location, chronological period, research sample (gender, age, etc.)
 
15. Rights Copyright and permissions Copyright (c) 2018 Journal of Applied Surfaces and Interfaces